Advances in Organometallic Chemistry, 7 by F G A Stone; Robert West

By F G A Stone; Robert West

ADVANCES ORGANOMETALLIC CHEMISTRY V 7.

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Nonmetal Hydrides . C. Hydrogen Halides and Other Proton Acids D. Metal Halides . E. Alkyl and Acyl Halides . F. Halogens . G. Pseudohalogens . V. Addition-Elimination Reactions . VI. Examples in Homogeneous Catalysis . A. Hydrogenation . B. Hydroformylation . C. Decarbonylation . D. Ethylene Dimerization . References . . . . . . . . . . . . . * * * * * .

Thieme, Stuttgart, Germany, 1968. Oxidative=Addition Reactions of d8 Complexes JAMES P. COLLMAN' Department of Chemistry, University of North Carolina Chapel Hill, North Carolina W A R R E N 'R. ROPER Department of Chemistry, University of Auckland Auckland. New Zealand I. Introduction . . 11. Mechanisms . A. Kinetic Studies . B. Stereochemistry . 111. Intermediate Examples . A. Oxygen Complexes . B. Olefin Complexes . C. Acetylene Complexes . IV. Examples of Oxidative-Addition Reactions A. Hydrogen .

H. Attwell, 1,1,2-triphenyl-l-silacyclobutaneand 1,1,2-triphenyl-l -silacyclopentane, in order to compare the reactivities of these two compounds. The five-membered ring was found to be quite unreactive under conditions where the four-membered ring was readily cleaved. Mechanisms involving d-orbital participation should be operative in cleavage of both compounds. T h e observed difference in reactivity between the two cyclic compounds can be explained in part by a qualitative consideration of both the ground and the transition state energies.

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